I play a druid that has charm soloed for most of my levels. What seems to be happening to me is that mobs well below your level, like 5+ levels below you, will rarely break early.
Mobs close to, but below your level, will break early most of the time, but are usually good for killing 1-2 other monsters before they break. These monsters I have found charisma boosting items to help with. Getting my cha from 75 to 105 has a noticeable effect on my charm duration with mobs just under my lvl.
Charming equal or higher level mobs they last a couple of seconds no matter what you do with your charisma.
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