There are no animals in Velks, so charming is out. My guess is the large outdoor zones have some charming or quadding that you can do, but I don't have any real experience doing it myself.
For XP though, mobs in velious just have higher hp. There are some good random drops and spawns, and you can probably sell skins, pelts etc. for a pretty penny. However, I don't personally know of any outdoor drops that are going to compete for cash with seafuries, nor with permafrost bear pits for xp.
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