#1 Stormfeather
#2 Scout Charisa
#3 Keldor (OOIV)
#4 Lodizal
Honorable mentions:
Vaniki
Myga
Vilefang
Master Yael
Oh, and if we're talking about late Velious -
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These dudes.
If you count raid mobs, priority is going to be ST Keys for the first few months. Tormax and Vulak follow them.